1, Nature Materials Cover: The use of “phagocytosis” synthesis of functional colloidal particlesUniversity of Bristol Stephen Mann (author) and other people inspired by cell phagocytosis, the preparation of self-driven magnetic Pickering emulsion (MPE), can be selective intake of silica gel particles. After the intake of colloidal particles can selectively transmit and release this water-soluble carrier, while MPE droplets can also be coupled within the enzyme activity. This provides a revelation for the development of colloidal-based new materials and provides a new micrometer-scale regulation for particle synthesis to induce highly ordered behavior.Phagocytosis-inspired behaviour in synthetic protocell communities of compartmentalized colloidal objects(Nature Materials,2017,Doi:10.1038/nmat4916)2, Nature Nanotechnology Cover: Sulfated Glycopeptide Nanostructures are used to activate multifunctional proteins North American University Samuel I. Stupp (Correspondent) et al. Reported supramolecular sulfated glycopeptide nanostructures that extend the signal of bone morphogenetic protein 2 more naturally than the natural sulfated polysaccharide heparin, which promotes Spinal bone regeneration, although far less animal model, but this bioactive nano-structure in the future involved in the field of protein research will have more applications possible.Sulfated glycopeptide nanostructures for multipotent protein activation(Nature Nanotechnology,2017,Doi:10.1038/nnano.2017.109)3, Nature Chemistry Cover: Polyamide-nickel metal polymer University of Bristol Ian Manners (author) and others using the two nickel-nickel monomer through the ring-opening polymerization to form the main chain of poly-nickel-nickel-containing metal polymer, nickel-nickel monomer due to its relatively weak nickel – The interaction between static and dynamic can be converted between each other. At the same time, the study found that the system in the lower concentration, increase the temperature or the existence of a polar solvent, will make poly-lignocene polymerization. The synthetic magnetic material has the potential for data storage and retrieval.Main-chain metallopolymers at the static–dynamic boundary based on nickelocene(Nature Chemistry,2017,Doi:10.1038/nchem.2743)4, JACS cover: reduce the conjugate polymer single, tri-state energy difference universal method Andrew J. Musser and Richard H. Friend of the University of Cambridge and Hugo Bronstein (co-author of the University of London), who introduced a universal method to reduce the single, tri-state energy difference in conjugated polymers, And the receptors are orthogonally connected to spatially separate electrons and holes. This method allows the conjugated polymer to greatly reduce the exchange energy, promote the formation of triplet and thermally excited delayed fluorescence, the mechanism of these two processes through the excited state π – π * and charge transport between the mixed drive.Synthesis and Exciton Dynamics of Donor-Orthogonal Acceptor Conjugated Polymers: Reducing the Singlet–Triplet Energy Gap(JACS,2017,DOI: 10.1021/jacs.7b03327)5, JACS cover: Cu-Oxo cluster catalyzes methane oxidation University of Munich, Johannes A. Lercher (author) et al. Used atomic layer deposition to deposit copper oxides on the metal nodes of MOF NU-1000, which catalyze the oxidation of methane under mild conditions to produce methanol, Selectivity to 45-60%. The Cu-oxo supported on the MOF is an atomic cluster formed by several Cu atoms and is mixed at about 15% Cu + and 85% Cu2 + under atmospheric conditions.Methane Oxidation to Methanol Catalyzed by Cu-Oxo Clusters Stabilized in NU-1000 Metal–Organic Framework(JACS,2017,DOI: 10.1021/jacs.7b02936)6, Angew. Chem. Int. Ed. Cover: Interactions between aromatic-perfluoro aromatic and charge transport in organic concentrating systems (Pyrene-OFN) and pyrene-TCNB were synthesized by supramolecular self-assembly of two typical luminescent organic eutectic pyrene-pyrene-OFNs. It was found that the two intergranular interaction modes exhibited different optical properties, namely, aromatic-perfluoro aromatic (AP) and charge transport (CT) interactions. And the competitive relationship between these two different molecules can be used to produce more complex organic concentrating systems.Competition between Arene–Perfluoroarene and Charge-Transfer Interactions in Organic Light-Harvesting Systems(Angew. Chem. Int. Ed.,2017,DOI: 10.1002/anie.201702084)7, Angew. Chem. Int. Ed. Cover: Transparent hollow micrometer for improved nonlinear photoluminescence bit selectivityHong Kong City University Feng Wang (Correspondent) et al. Prepared a one-dimensional hollow micrometer structure by kinetic control of the crystal growth process, and synthesized the hexagonal NaYbF4 micrometer rods along the longitudinal axis by hydrothermal method. At the same time, from the light scattering and reflection of the inner wall of mutual interference can be achieved through the micro-rods to control the optical density.Crystalline Hollow Microrods for Site-Selective Enhancement of Nonlinear Photoluminescence(Angew. Chem. Int. Ed.,2017,DOI: 10.1002/anie.201703600)8, Adv. Mater. Cover: Ultra-thin Bi5O7Br nanotube light reduction N2 Professor Chen Hao of Huazhong Agricultural University and Prof. Ye Jinhua, a member of the National Institute of Materials Science, Japan, jointly synthesized the Bi5O7Br nanotubes with a diameter of 5 nm. This material has a strong nanotube structure, a suitable absorption limit and exposed Many surface sites help to provide sufficient visible light-induced oxygen vacancies to achieve the reduction of N2 light in the atmosphere into pure water.Light-Switchable Oxygen Vacancies in Ultrafine Bi5O7Br Nanotubes for Boosting Solar-Driven Nitrogen Fixation in Pure Water(Adv. Mater.,2017,DOI: 10.1002/adma.201701774)9, Adv. Mater. Cover: High power conversion efficiency of WSe2-MoS2 p-n heterojunction solar cells Lih-Juann Chen, National Tsinghua University, and Jr-Hau He (co-author), King Abdullah University of Science and Technology, et al. Prepared a continuous growth of non-alloyed 2D single-layer WSe2-MoS2 pn heterojunctions and studied their photovoltaic properties , In the AM 1.5G lighting, the material showed a power conversion efficiency of 2.56%. The large surface area allows the barrier area to be completely exposed, resulting in excellent omnidirectional light collection characteristics with an efficiency of only 5% when the incident angle is as high as 75 °.Single Atomically Sharp Lateral Monolayer p-n Heterojunction Solar Cells with Extraordinarily High Power Conversion Efficiency(Adv. Mater.,2017,DOI: 10.1002/adma.201701168)10, Adv. Energy Mater. Cover: Single Layer Silicon Embedded Graphite for Lithium Ion BatteriesA single layer Si embedded graphite / carbon mixed electrode (G / SGC) was prepared by Minseong Ko and Jaephil Cho (co-author of the National Institute of Science and Technology), Korea. And the electrodes were compared with commercially available materials under the same conditions. Because SGC has a good compatibility with traditional graphite, and SGC structural characteristics are also very good to determine, so there is a potential application prospects. This also contributes to the research and development of high-energy lithium-ion battery Si-based anode materials.One-to-One Comparison of Graphite-Blended Negative Electrodes Using Silicon Nanolayer-Embedded Graphite versus Commercial Benchmarking Materials for High-Energy Lithium-Ion Batteries(Adv. Energy Mater.,2017,DOI: 10.1002/aenm.201700071)
Quelle: Meeyou Carbide

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